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Jobin Yvon, Triax 550 monochromator (250nm-1800nm)
Melles Griot single mode Ar+ Laser (488nm)
ARS 202N Closed Cycle Refrigerator System (5.5-350K)
Photomultiplier tube and other UV-IR photodetectors
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Photoluminescence
Spectroscopy
Photoluminescence spectroscopy is a contactless, nondestructive
method of probing the electronic structure of materials. Specifically,
light is directed onto a sample, where it is absorbed and imparts
excess energy into the material in a process called "photo-excitation."
One way this excess energy can be dissipated by the sample is
through the emission of light, or luminescence. In the case
of photo-excitation, this luminescence is called photoluminescence.
The intensity and spectral content of this photoluminescence
is a direct measure of various important material properties.
More specifically, photo-excitation causes electrons within
the material to move into permissible excited states. When these
electrons return to their equilibrium states, the excess energy
is released and may include the emission of light (a radiative
process) or may not (a nonradiative process). The energy of
the emitted light-or photoluminescence-is related to the difference
in energy levels between the two electron states involved in
the transition-that is, between the excited state and the equilibrium
state. The quantity of the emitted light is related to the relative
contribution of the radiative process.
Photoluminescense
Applications:
" Band gap determination. The most common radiative transition
in semiconductors is between states in the conduction and valence
bands, with the energy difference being known as the band gap.
Band gap determination is particularly useful when working with
new compound semiconductors.
" Impurity levels and defect detection. Radiative transitions
in semiconductors also involve localized defect levels. The
photoluminescence energy associated with these levels can be
used to identify specific defects, and the amount of photoluminescence
can be used to determine their concentration.
" Recombination mechanisms. As discussed above, the return
to equilibrium, also known as "recombination," can
involve both radiative and nonradiative processes. The amount
of photoluminescence and its dependence on the level of photo-excitation
and temperature are directly related to the dominant recombination
process. Analysis of photoluminescence helps to understand the
underlying physics of the recombination mechanism.
" Material quality. In general, nonradiative processes
are associated with localized defect levels, whose presence
is detrimental to material quality and subsequent device performance.
Thus, material quality can be measured by quantifying the amount
of radiative recombination.
Special
Features:
" Various excitation wavelengths allow for varying penetration
depths into the material, and thus, varying levels of volume
excitation.
" Sensitivity down to the level of parts per thousand,
depending on impurity species and host.
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